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Redox Metal-Ligand Cooperativity Enables Robust and Efficient Water Oxidation Catalysis at Neutral pH with Macrocyclic Copper Complexes

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dc.contributor.affiliation"Institute of Chemical Research of Catalonia (ICIQ), Barcelona Institute of Science and Technology (BIST), Avinguda Països Catalans, 16, Tarragona, 43007, Spain"," Instituto Madrileño de Estudios Avanzados en Nanociencia (IMde A Nanociencia), Calle Faraday, 9, Madrid, 28049, Spain"," Departament de Química, Universitat Autònoma de Barcelona, Bellaterra, 08193, Spain"en
dc.contributor.affiliation000000041762408X
dc.contributor.authorGarrido-Barros P.
dc.contributor.authorMoonshiram D.
dc.contributor.authorGil-Sepulcre M.
dc.contributor.authorPelosin P.
dc.contributor.authorGimbert-Suriñach C.
dc.contributor.authorBenet-Buchholz J.
dc.contributor.authorLlobet A.
dc.date.accessioned2020-12-04T11:40:17Z
dc.date.available2020-12-04T11:40:17Z
dc.date.issued2020
dc.identifier.doi10.1021/jacs.0c06515en
dc.identifier.urihttp://hdl.handle.net/20.500.12614/736
dc.journal.titleJournal of the American Chemical Societyen
dc.language.isoenen
dc.page.initial17434en
dc.relation.projectIDTEMPSupport from MINECO, FEDER, and AGAUR is gratefully acknowledged (CTQ2016-80058-R, SEV-2013-0319, ENE2016-82025-REDT, CTQ2016-81923-REDC, and 2017-SGR-1631). P.G.-B acknowledges the “La Caixa” Foundation for the Ph.D. grant. D.M. acknowledges support from the Severo Ochoa Excellence program (SEV-2016-0686) from the Instituto IMDEA Nanociencia Acciones de Dinamization Europa Investigacion grant (EIN2019-103399), and the “Ministerio de Ciencia, Innovacion y Universidades Grant” (PID2019-111086RA-I00). XAS experiments were performed at the CLAESS beamline at ALBA Synchrotron with the beamline support of the ALBA staff under proposal no. 2016091818 and additionally used resources of sector 20 beamline at the Advanced Photon Source (APS) at Argonne National Laboratory. Sector 20 beamline at APS is operated by the U.S DOE, under contract no. DE-AC02-06CH11357 and the Canadian Light Source.
dc.rightsAtribución-NoComercial-SinDerivadas 3.0 España*
dc.rights.accessRightsopen accessen
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/3.0/es/*
dc.titleRedox Metal-Ligand Cooperativity Enables Robust and Efficient Water Oxidation Catalysis at Neutral pH with Macrocyclic Copper Complexesen
dc.typeresearch articleen
dc.volume.number142en
dspace.entity.typePublication

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