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S. A. S. and N. A. acknowledge funding from the European Commission through the FP7 ITN MOLESCO (Project Number 606728). E. A. gratefully acknowledges financial support from L?Or?al-UNESCO through the Women in Science program. A. J. M.-M. acknowledges the financial support from MICINN (Spain) through the scholarship BES-2012-057346. D. Y. and T. S. acknowledge the support from the Ministry of Science and Technology of the Republic of China under the MOST 104-2112-M-018-004 and 104-2221-E-018-017. D. P. is thankful for funding from the Spanish Ministry of Economy and Competitiveness through FIS2015-67367-C2-1-P. R. F. thanks the Netherlands Organisation for Scientific Research (NWO) for the financial support through the research programme Rubicon with the project number 680-50-1515. AC-G. acknowledges the support from the BBVA Foundation through the fellowship ?I Convocatoria de Ayudas Fundacion BBVA a Investigadores, Innovadores y Creadores Culturales? (?Semiconductores ultradelgados: hacia la optoelectronica flexible?), from the MINECO (Ram?n y Cajal 2014 program, RYC-2014-01406), from the MICINN (MAT2014-58399-JIN) and from the Comunidad de Madrid (MAD2D-CM Program (S2013/MIT-3007)), and the European Commission under the Graphene Flagship, contract CNECTICT-604391.
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S. K. wishes to acknowledge funding from the European Union's Horizon 2020 research and innovation programme under the Marie Skłodowska-Curie grant agreement No 663830. Financial support was also provided by the Reducing Industrial Carbon Emissions (RICE) operation part-funded by the EU's European Regional Development Fund through the Welsh Government . The authors also acknowledge the assistance provided by the Swansea University AIM Facility, funded in part by the EPSRC (EP/M028267/1), the European Regional Development Fund through the Welsh Government (80708) and the Sêr Solar project via the Welsh Government . Use of the TAMU Materials Characterization Facility and Dr. Wilson Serem are acknowledged.
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S. L. and E. M. P. gratefully acknowledge funding from the European Research Council MINT (ERC-StG-2012-307609), the MINECO of Spain (CTQ2014-60541-P) and the Comunidad de Madrid (MAD2D project, S2013/MIT-3007). Y. P. and A. R. acknowledge financial support from the European Research Council (ERC-2010-AdG-267374), Spanish grant (FIS2013-46159-C3-1 P), Grupos Consolidados (IT578-13), and AFOSR Grant No. FA2386-15-1-0006 AOARD 144088 H2020-NMP-2014 project MOSTOPHOS, GA no. SEP-210187476 and COST Action MP1306 (EUSpec), as well as technical and human support provided by IZO-SGI SGIker of UPV/EHU and its European funding (ERDF and ESF).
1
S. M. P. acknowledges financial support from a postdoctoral contract of the Regional Government of Madrid (Spain) (Grant PEJD-2016/IND-3217). D. V. C. thanks a contract from Spanish MINECO under the FPI predoctoral program. This work has been financed by the Spanish MINECO (Grant CTQ2015-65033-P) and the Spanish Ministry of Science and Innovation (Grant PGC2018-096444-B-I00). This research has been carried out within the Unidad Asociada Qú?mica Física Molecular between the Departa-mento de Qú?mica Física of Universidad Complutense de Madrid and CSIC. The facilities provided by the Centro de Láseres Ultra-rrápidos at Universidad Complutense de Madrid are gratefully acknowledged. The Centro de Supercomputación de Galicia (CESGA, Spain) and the Centro Técnico de Informática (CTI, CSIC) are acknowledged for the use of their resources.
1
S. Oberli and A. Picón acknowledge funding from Comunidad de Madrid through TALENTO grant ref. 2017-T1/IND-5432. F. Martín and J. González-Vázquez acknowledge the MINECO projects FIS2016-77889-R. F. Martín acknowledges the Severo Ochoa Programme for Centres of Excellence in R&D (SEV-2016-0686) and the María de Maeztu Programme for Units of Excellence in R&D (MDM-2014-0377).
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S.D.-T. gratefully acknowledges the Juan de la Cierva program of the Spanish Ministerio de Educación y Ciencia. We acknowledge a generous allocation of computer time at the Centro de Computación Cientfica at the Universidad Autónoma de Madrid (CCC-UAM). This work was supported by the DGI Projects FIS2007-60064 and CSD 2007-00010, and the CAM project S2009/MAT1726.
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S.D.S.F. acknowledges the economic support by CONACyT and Instituto Politécnico Nacional SIP 20180252 (México). The authors thank the Laboratorio Nacional de Conversión y Almacenamiento de Energía (LNCAE) for access to its experimental facility. This research was partially funded by the Spanish Ministry of Economy and Competitiveness under grant MAT2017-88148-R (AEI/FEDER, UE) and by the Spanish Ministry of Science, Innovation and Universities (MCIU) through projects PGC2018-096016-B-I00 (MCIU/AEI/FEDER to L.G.) and PID2019-106301RB-I00 (G.S.). The microscopy works were conducted at the Advanced Microscopy Laboratory from the Servicio General de Apoyo a la Investigación-SAI, Universidad de Zaragoza.
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S.H, C.C, L.G., and U.K. acknowledge support by the ERC advanced Grant No. ERC-2012-ADG-20120216 within the seventh framework program of the European Union and by the NCCR MUST, funded by the Swiss National Science Foundation. M.L. acknowledges support from the ETH Zurich Postdoctoral Fellowship Program. A J.G., L.A., and F.M. acknowledge the support from the European Research Council under the ERC Grant No. 290853 XCHEM, from the European COST Action No. CM1204 XLIC, the MINECO Project No. FIS2013-42002-R, the ERA-Chemistry Project No. PIM2010EEC- 00751, and the European Grant No. MC-ITN CORINF. Calculations were performed at the Centro de Computacian Cient?-fica of the Universidad Autonoma de Madrid (CC-UAM) and the Barcelona Supercomputing Center (BSC). I.I. and A.S.K. acknowledge support of the Australian Research Council (Grant No. DP120101805) and the use of the National Computational Infrastructure Facility. J.M.D. acknowledges support from the Swedish Research Grants No. 2013-344 and No. 2014-3724. E.L. acknowledges support from the Swedish Research Council, Grant No. 2012-3668. Moreover, this research was supported in part by the Kavli Institute for Theoretical Physics (National Science Foundation under Grant No. NSF PHY11-25915) and by NORDITA, the Nordic Institute for Theoretical Physics.
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S.J.S. acknowledges support from the Air Force Office of Scientific Research Grant No. FA9550-15-1-0428, and the Material Research Science and Engineering Center at the University of Chicago, No. NSF-DMR-14-20709. F.M., C.D., A.S.M., and M.d.C. acknowledge the MICINN Project No. FIS2013-42002-R, CAM Project No. S2014/MIT-2850, NANOFRONTMAG, and the CCC-UAM and the University of Chicago Research Computing Center for allocation of computer time. C.D. acknowledges the MICINN Project No. CTQ2013-50150-EXP and the Ramon y Cajal program. A.S.M. and M.d.C. acknowledge the FPI program of the MICINN, co-financed by the E.S.F. N.T.P. acknowledges a National Science Foundation Graduate Research Fellowship. N.S.L. acknowledges support from the National Science Foundation (Grant No. CHE-1214152), and research was in part carried out at the Molecular Materials Research Center of the Beckman Institute of the California Institute of Technology.
1
S.K.C. acknowledges Programme International de Coopération Scientifique (PICS) du CNRS under Grant No. 6161 and SIMEM Doctoral School at Universite de Caen Normandie for financial support. IMDEA-Nanociencia acknowledges support from the “Severo Ochoa” Program for Centres of Excellence in R&D (MINECO, Grant No. SEV-2016-0686). F.A., J.C., and P.P. acknowledge the support of Spanish MINECO Project Nos. FIS2015-67287-P and FIS2016-78591-C3-1-R and the Comunidad de Madrid through Project NANOFRONTMAG CM. This project has received funding from the European Union’s Horizon 2020 research and innovation programme under Grant Agreement Nos. 737116 (byAxon) and 654360 NFFA-Europe.
1
S.M. is grateful to the TUT postdoctoral programme. T.T. is grateful for the financial support of the MINECO, Spain (CTQ2017-85393-P), the Comunidad de Madrid (FOTO-CARBON, S2013/MIT-2841). IMDEA Nanociencia acknowledges support from the ‘Severo Ochoa’ Programme for Centres of Excellence in R&D (MINECO, Grant SEV-2016-0686).
1
S.P. and J.V. acknowledge the support of the Agence Nationale de la Recherche, Project ANR-14-CE26-0012 (ULTRASKY). B. Fernandez, Ph. David, and E. Mossang are acknowledged for their technical help. D.S.C was supported by a CNPq Scholarship (Brazil). F.A. acknowledges the support of Spanish MINECO for exchange Grant No. EEBB-I-16-11844. P.P., R.G., A.G., and J.C. acknowledge the support of Spanish MINECO Project No. FIS2016-78591-C3-1-R (SKYTRON). F.A., P.P., and J.C. acknowledge the support of the Comunidad de Madrid through Project NANOFRONTMAG CM.
1
SP acknowledges Science and Engineering Research Board (ECR/2017/002433) and IIT Delhi for funding. D. M. acknowledges funding from the Severo Ochoa Excellence program (SEV-2016-0686) from the Instituto IMDEA Nanociencia, the Acciones de Dinamización “Europa Investigacion” grant (EIN2019-103399), and the Spanish Ministerio de Ciencia, Innovacion y Universidades grant (PID2019-111086RA-I00). The research leading to part of the results was further supported by the project CALIPSOplus under the Grant Agreement 730872 from the EU Framework Programme for Research and Innovation HORIZON 2020. We also thank Dr Wolfgang Caliebe for help with experiments at the Petra P64 beamline at DESY, a member of the Helmholtz Association (HGF) (Germany). The DFT calculations (SI) were performed in the Scientic Computing Center-Autonomous University of Madrid (CatDesignProject, PI: D. Moonshiram), thanks to CPU time and other resources granted by the institution. We acknowledge Prof. Kaushik Ghosh, IIT Roorkee for helping with EPR measurements. We thank Prof. Kuntal Manna, IIT Delhi for helping with GC-mass measurements. KK acknowledges MHRD for the fellowship. MB thanks SERB for the Inspire fellowship. GG thanks IIT Delhi for the Institute Post-Doctoral Fellowship.
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Spanish Ministry of Economy and Competitiveness [FIS2015–67765-R to F.J.C., BFU2012–31825, BFU2015– 63714-R to B.I.], National Institutes of Health [GM45925 to L.S.K.], Comunidad de Madrid [NanoMagCOST P2018 INMT-4321], Programa de Financiación Universidad Complutense de Madrid–Santander Universidades [CT45/15-CT46/15 to F.C.], Ministerio de Educación Cultura y Deporte [FPU2014/06867 to K.M.L.]. IMDEA Nanociencia acknowledges support from the Severo Ochoa Programme for Centers of Excellence in R&D [MINECO, Grant SEV-2016–0686]. Funding for open access charge: Spanish Ministry of Economy and Competitiveness [BFU2015-63714-R]. Conflict of interest statement. None declared.
1
Studies at MPI Stuttgart were supported by the European Science Foundation (ESF) EUROCORES-SONS2 programme FunSMARTs II. Work in Madrid was financed by the Spanish MICINN (projects FIS2007-61114, FIS2007-60064, NAN2004-08881-C02-01, CTQ2006-08558 and Consolider CSD2007-00010), the Comunidad de Madrid (projects S-0505-MAT-0194 and S2009/MAT-1726) and the European Union (‘MONET’ project, MEST-CT-2005-020908). R.O. thanks the MEC for salary support through the Ramón & Cajal programme. All the computations were performed at Mare Nostrum Barcelona Supercomputer Center and Centro de Computación Científica de la UAM.
1
Support from MINECO , FEDER , and AGAUR is gratefully acknowledged through grants CTQ2016-80058-R , CTQ2015-73028-EXP , SEV 2013-0319 , ENE2016-82025-REDT , CTQ2016-81923-REDC , and 2017-SGR-1631 . D.M. acknowledges funding from the Severo Ochoa ( SEV-2016-0686 ) Excellence Program from IMDEA Nanociencia. XAS experiments were performed at the CLAESS beamline at ALBA Synchrotron under proposal No. 20170913 and 2017032110.
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Support from MINECO, FEDER and AGAUR are gratefully acknowledged through grants CTQ2016-80058-R, CTQ2015-73028-EXP, SEV 2013-0319, ENE2016-82025-REDT, CTQ2016-81923-REDC, and 2017-SGR-1631. The work has further been supported by the University of Zurich, the University Research Priority Program “Solar Light to Chemical Energy Conversion” (LightChEC) and the Swiss National Science Foundation (grant. No. PP00P2 170667). Computational time by the Swiss national supercomputing center (accounts: s745 and s875) are gratefully acknowledged.
1
Support from MINECO, FEDER, and AGAUR is gratefully acknowledged (CTQ2016-80058-R, SEV-2013-0319, ENE2016-82025-REDT, CTQ2016-81923-REDC, and 2017-SGR-1631). P.G.-B acknowledges the “La Caixa” Foundation for the Ph.D. grant. D.M. acknowledges support from the Severo Ochoa Excellence program (SEV-2016-0686) from the Instituto IMDEA Nanociencia Acciones de Dinamization Europa Investigacion grant (EIN2019-103399), and the “Ministerio de Ciencia, Innovacion y Universidades Grant” (PID2019-111086RA-I00). XAS experiments were performed at the CLAESS beamline at ALBA Synchrotron with the beamline support of the ALBA staff under proposal no. 2016091818 and additionally used resources of sector 20 beamline at the Advanced Photon Source (APS) at Argonne National Laboratory. Sector 20 beamline at APS is operated by the U.S DOE, under contract no. DE-AC02-06CH11357 and the Canadian Light Source.
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Support is acknowledged from the Spanish MICINN (CTQ2011-24187/BQU and CONSOLIDER INGENIO 2010, CSD2007-00010 on Molecular Nanoscience) and the CAM (MADRISOLAR-2, S2009/PPQ/1533). EP would like to acknowledge the European Research Council starting Grant ERCstg-POLYDOT and the national projects CONSOLIDER HOPE 0007-2007 and MICINN CTQ-2007-60746-BQU as well as Catalonian regional government for the project 2009 SGR 207.
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Supported by Ministerio de Economía y Competitividad in Spain grants ( BIO2015-64221-R ( MINECO/AEI/FEDER UE ) and BFU2015-65625-P ( MINECO/FEDER UE ), Ministerio de Ciencia, Innovación y Universidades in Spain grant RTI2018-095624-B-C21 ( MCIU/AEI/FEDER UE ), Basque Government grant IT1196-19 , doctoral studentships to E.R., and a doctoral scholarship to A.G.V. ( FPU2016-01727 ). P.C. also acknowledges a research associate contract at the University of the Basque Country (DOCREC18/01) and a postdoctoral fellowship from the Basque Government ( POS_2018_1_0066 ). L.D. acknowledges ANII (Agencia Nacional de Investigación e Innovación) and the Institut Pasteur de Montevideo for funding his postdoctoral fellowship. We gratefully thank Unai Lorenzo-Sierra for developing the sFCS software and analysis algorithms.
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